Light-absorbing impurities (including black carbon, organic carbon, and mineral dust) deposited on snow can reduce surface albedo and contribute to the near-worldwide melting of snow cover and ice. This study found that the black carbon, organic carbon, and dust concentrations in snow cover ranged generally from 202–17 468 ng g<sup>−1</sup>, 491–13 880 ng g<sup>−1</sup>, and 22–846 µg g<sup>−1</sup>, respectively, with higher concentrations in the central to northern areas of the Third Pole region (referred to by scientists also as the Tibetan Plateau and its surrounding mountains). Footprint analyses suggested that the northern Third Pole was influenced mainly by air masses from Central Asia with some Euro-Asia influence; air masses in the central and Himalayan region originated mainly from Central and South Asia. The open burning-sourced black carbon contributions decreased from ~ 50 % in the southern Third Pole region to ~ 30 % in the northern Third Pole region. The contribution of black carbon and dust to snow albedo reduction reached approximately 37 % and 15 %, respectively. The effect of black carbon and dust reduced the average snow cover duration by 3.1 ± 0.1 days to 4.4 ± 0.2 days. Meanwhile, the black carbon and dust had an import implication for snowmelt water loss over the Third Pole region. Findings indicate that the impacts of black carbon and mineral dust need to be properly accounted for in future regional climate projections, particularly in the high-altitude cryosphere.